If you love Venezuelan arts and crafts then go to the town of Hatillo(maybe 30 minutes from El Centro). There is a shop there called Hansi. It has handcrafted items from all over Venezuela in one place. The town itself is beautiful.
It's a small town but very cozy.
There are several handicraft shops with the nicest things!
The day I was there there were some performers in the Plaza Bolivar....
And seemed like a very family thing to do on Sundays, just to hang out on the square, have some coffee in the nearby cafés...
El Hatillo is a small village only a short drive from Caracas centre. This quiet place is a part of the city.